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Electronic textiles (e‐textiles) are in prime position to revolutionize the field of wearable electronics owing to their ubiquitous use and universal acceptance. However, mechanical incompatibility between the rigid conductive components on the soft textile platforms creates fragile e‐textile systems with poor electromechanical attributes. In this work, a novel design strategy to inkjet print reactive silver inks onto woven textiles with Kirigami‐inspired patterning to create e‐textiles with enhanced electromechanical features is introduced. By controlling the print processing and curing conditions, uniform conductive coatings with sheet resistances of 0.09 Ω sq⁻¹are achieved such that they do not interfere with the textiles innate flexibility, breathability, comfort, and fabric hand. The electromechanical coupling of the printed textiles shows a direct dependence on the anisotropic nature of the woven structures. Introducing Kirigami patterning creates robust devices that enhance and stabilize the electrical conductivity (ΔR/R₀< −20%) over large strain regimes (>150%). Furthermore, an electrocardiogram monitoring system fabricated from Kirigami e‐textiles exhibits stable signal acquisition under extreme deformations from arm joint flexion. The distinct properties of Kirigami patterning on e‐textiles enable unprecedented electromechanical performance in wearable textile electronics.

In this work, a novel technique of inkjet printing e‐textiles with particle free reactive silver inks on knit structures is developed. The inkjet‐printed e‐textiles are highly conductive, with a sheet resistance of 0.09 Ω sq^‐1, by means of controlling the number of print passes, annealing process, and textile structures. It is notable that the inkjet process allows textiles to maintain its inherent properties, including stretchability, flexibility, breathability, and fabric hand after printing process. This is achieved by formation of ultrathin silver layers surrounding individual fibers. The silver layers coated on fibers range from 250 nm to 2.5 µm, maintaining the size of interstices and flexibility of fibers. The annealing process, structure of fibers, and printed layers significantly influence the electrical conductivity of the patterned structures on textiles. Outstanding electrical conductivity and durability are demonstrated by optimizing print passes, controlling textile structures, and incorporating an in situ annealing process. The electrical resistance dependence on the strain rate of the textiles is examined, showing the ability to maintain electrical conductivity to retain light‐emitting diode use, stable more than 500 consecutive strain cycles. Most importantly, inkjet‐printed e‐textiles maintain their characteristic washability, breathability, and fabric hands for applications in wearable technology.